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Yin et al 2019, Water nanostructure formation on oxide probed.pdf2,03 MBAdobe PDFView/Open
Title: Water nanostructure formation on oxide probed in situ by optical resonances
Authors: Yin, Y.Wang, J.Wang, X.Li, S.Jorgensen, M.R.Ren, J.Meng, S.Ma, L.Schmidt, O.G.
Publishers Version: https://doi.org/10.1126/sciadv.aax6973
Issue Date: 2019
Published in: Science Advances Vol. 5 (2019), No. 10
Publisher: Washington : American Association for the Advancement of Science (A A A S)
Abstract: The dynamic characterization of water multilayers on oxide surfaces is hard to achieve by currently available techniques. Despite this, there is an increasing interest in the evolution of water nanostructures on oxides to fully understand the complex dynamics of ice nucleation and growth in natural and artificial environments. Here, we report the in situ detection of the dynamic evolution of nanoscale water layers on an amorphous oxide surface probed by optical resonances. In the water nanolayer growth process, we find an initial nanocluster morphology that turns into a planar layer beyond a critical thickness. In the reverse process, the planar water film converts to nanoclusters, accompanied by a transition from a planar amorphous layer to crystalline nanoclusters. Our results are explained by a simple thermodynamic model as well as kinetic considerations. Our work represents an approach to reveal the nanostructure and dynamics at the water-oxide interface using resonant light probing.
Keywords: Light emission; Morphology; Nanoclusters; Resonance; Resonators; Artificial environments; Critical thickness; Dynamic characterization; Dynamic evolution; In-situ detections; Nanostructure formation; Thermodynamic model; Water-oxide interface; Quantum optics
DDC: 530
License: CC BY 4.0 Unported
Link to License: https://creativecommons.org/licenses/by/4.0/
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